Environmentally sustainable lithium-ion battery cathode binders based on cellulose nanocrystals

Huang, Xingkang; You, Haoyang; Yan, Xiaoli; Borkiewicz, Olaf J.; Wiaderek, Kamila M.; Hui, Janan; Hersam, Mark C.; Chaudhuri, Santanu; Rowan, Stuart J.; Chen, Junhong

Huang, Xingkang; You, Haoyang; Yan, Xiaoli; Borkiewicz, Olaf J.; Wiaderek, Kamila M.; Hui, Janan; Hersam, Mark C.; Chaudhuri, Santanu; Rowan, Stuart J.; Chen, Junhong

2024

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Abstract

Aqueous binders as environmentally sustainable alternatives to conventional polyvinylidene difluoride (PVDF) binders have not yet been successful for cathodes in lithium-ion batteries (LIBs). Here, carboxylic acid functionalized cellulose nanocrystals (CNC-COOHs) have been obtained from Miscanthus × giganteus (M×G) biomass and evaluated as aqueous binders for LIB cathodes.

Details

Title

Environmentally sustainable lithium-ion battery cathode binders based on cellulose nanocrystals

Author

Huang, Xingkang : University of Chicago : (https://orcid.org/0000-0001-7965-1866)
You, Haoyang : University of Chicago : (https://orcid.org/0000-0001-7462-2118)
Yan, Xiaoli : University of Illinois Chicago
Borkiewicz, Olaf J. : Argonne National Laboratory
Wiaderek, Kamila M. : Argonne National Laboratory
Hui, Janan : Northwestern University
Hersam, Mark C. : Northwestern University : (https://orcid.org/0000-0003-4120-1426)
Chaudhuri, Santanu : University of Illinois Chicago
Rowan, Stuart J. : University of Chicago : (https://orcid.org/0000-0001-8176-0594)
Chen, Junhong : University of Chicago : (https://orcid.org/0000-0002-2615-1347)

Content Type

Article

Published in

Journal of Materials Chemistry A

Identifier(s)

DOI: https://doi.org/10.1039/D4TA03305A

Data availability statement

The data supporting this article have been included as part of the electronic supplementary information.

Funding Information

National Science Foundation, MADE-PUBLIC Future Manufacturing Research Grant Program, CMMI-2037026

Publication Date

2024-08-16