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Abstract
Designing materials with specific properties has been a long-time goal of the physics community.
Optical photons have recently emerged as a promising candidate for such metamaterials
due to their fast dynamics and available manipulation toolkit. In conjunction with carefully
engineered optical resonators, it is possible to precisely control the properties of individual
photons through the resonator Hamiltonian. The only missing ingredient to photonic
materials is strong photon-photon interactions.
This thesis describes the characterization of cavity Rydberg polaritons and the emergence
of strong interactions in such a system. Electromagnetically induced transparency (EIT) is
used to create quasiparticles that inherit the properties of both photons and Rydberg atoms:
fast dynamics and trapping from the photons and long-range dipole-dipole interactions from
the Rydberg atoms. The emergent polaritonic properties are characterized and controlled
through the dark-state rotation angle and agree very well with theoretical predictions.
We then expand upon this understanding of polaritons by putting them inside a zerodimensional
quantum dot. Confining the polaritons in such an object allows for strong
interparticle interactions to manifest. We observe these interactions through the temporal
auto-correlation intensity function g2(t) and verify the dimensionality of the quantum dot
itself by measure the polariton Rabi oscillations.
With the experimental demonstration of strong photonic interactions, a complete understanding
of Rydberg atoms and polaritons is needed to allow for better control of the system.
To this effect, the properties of Rydberg atoms are analytically and numerically understood
and the full formalism needed to describe resonator Rydberg polaritons is developed, along
with their interactions and various sources of decoherence. Furthermore, a renormalized
effective field theory for single mode cavities is developed and tested against full numerical
models, paving the way for the simulation of the physical phenomena of manybody states in
multi-mode cavities.
Strongly interacting cavity polaritons can be utilized in quantum gate and repeater protocols
for quantum information processing. Furthermore, combining the experimental and
theoretical work here with non-planar resonators presents a clear path to non-trivial topological
synthetic materials and strongly correlated quantum states.