Control of liquid crystals combining surface acoustic waves, nematic flows, and microfluidic confinement

Vásquez-Montoya, Gustavo A.; Emeršič, Tadej; Atzin, Noe; Tavera-Vázquez, Antonio; Mozaffari, Ali; Zhang, Rui; Guzmán, Orlando; Snezhko, Alexey; Nealey, Paul F.; de Pablo, Juan J.

doi:10.6082/rzaed-66a51

Published December 14, 2023 | Version v1

Journal article Open

Control of liquid crystals combining surface acoustic waves, nematic flows, and microfluidic confinement

1. University of Chicago
2. Hong Kong University of Science and Technology
3. Universidad Autónoma Metropolitana Iztapalapa
4. Argonne National Laboratory

The optical properties of liquid crystals serve as the basis for display, diagnostic, and sensing technologies. Such properties are generally controlled by relying on electric fields. In this work, we investigate the effects of microfluidic flows and acoustic fields on the molecular orientation and the corresponding optical response of nematic liquid crystals. Several previously unknown structures are identified, which are rationalized in terms of a state diagram as a function of the strengths of the flow and the acoustic field. The new structures are interpreted by relying on calculations with a free energy functional expressed in terms of the tensorial order parameter, using continuum theory simulations in the Landau-de Gennes framework. Taken together, the findings presented here offer promise for the development of new systems based on combinations of sound, flow, and confinement.

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