Quantum Information Processing with Dual-Species Atom Arrays

Over the past decade, quantum information science has progressed from few-qubit demonstrations to experiments with hundreds of qubits. Neutral atom processors based on individual atoms trapped in arrays of optical tweezers have emerged as a leading candidate due to their inherent scalability and flexible connectivity. Advanced protocols like measurement-based state preparation and quantum error correction, however, require efficient crosstalk-free mid-circuit operations for the readout, reset, and replenishment of a subset of qubits. In typical single-species atom arrays, where all atoms are identical and on-resonance, such operations necessitate complex overheads from single-site addressing, coherent transport, or shielding techniques, to mitigate the qubit decoherence induced from photons scattered by neighboring atoms. To address this challenge of engineering scalable quantum architectures compatible with efficient control techniques, we introduce and implement the first dual-species atom array platform, and explore new dynamics inaccessible in single-species arrays. In this approach, two atomic species are addressed independently due to the spectral separation between their control wavelengths. We engineer two-dimensional arrays from individual rubidium (Rb) and cesium (Cs) atoms in up to 512 optical tweezers, and show that the two species can be independently trapped, cooled, and imaged with state-of-the-art performance metrics. Harnessing this intrinsic crosstalk-free control, we establish the key primitives of mid-circuit readout, real-time processing and feed-forward, and coherent mid-circuit reloading. By integrating these capabilities, we realize in-sequence, real-time correction of correlated phase errors via a spectator qubit protocol. Next, we excite atoms to Rydberg states in the Förster regime, accessing hitherto unobserved enhanced interspecies Rydberg interactions, and program them to implement the first interspecies CNOT gate. We combine this multispecies entanglement with mid-circuit readout to achieve quantum non-demolition measurement of a Rb-qubit using an auxiliary Cs-qubit, circumventing physical qubit transport. Finally, leveraging the two qubit modalities, we present the first experimental demonstration of quantum cellular automata in atom arrays using only global addressing, and prepare a 17-qubit Cs cluster state with Rb-mediated interactions. The dual-species platform and techniques established in this thesis pave the way toward measurement-based algorithms and real-time feedback control in large-scale quantum systems.